研究内容
「材料の新大陸を切り拓く」をビジョンに掲げ、次世代エネルギー・エレクトロニクスを支える革新的な熱・電子・光機能材料の開発とデバイス応用に関する研究を行っています。
次世代パワーエレクトロニクス・光デバイス材料の開発
大電力を効率的に制御・変換できるパワーデバイスの重要性がますます高まっており、その実現には大きなバンドギャップをもつ半導体の開発が不可欠です。また、自動運転技術や医療・環境計測の発展には、高感度な光センサーに向けた半導体の開発が求められています。これらの次世代電子デバイスの性能革新を目指し、第一原理計算を活用した材料設計と薄膜成長技術を駆使して、新規半導体材料の開発に取り組んでいます。例えば、バンドギャップが4.7 eVの非平衡相ルチル型GeO2の薄膜成長とp型・n型制御や、層状半導体を基盤とする光センサー用半導体の開発などを進めています。

【記事・プレスリリース】
【関連論文】
Keisuke Ide, Naoto Watanabe, Takayoshi Katase, Masato Sasase, Junghwan Kim, Shigenori Ueda, Koji Horiba, Hiroshi Kumigashira, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Applied Physics Letters, vol. 121, iss. 19, pp. 192108, 2022.
@article{nokey,
title = {Low-temperature-processable amorphous-oxide-semiconductor-based phosphors for durable light-emitting diodes},
author = {Keisuke Ide and Naoto Watanabe and Takayoshi Katase and Masato Sasase and Junghwan Kim and Shigenori Ueda and Koji Horiba and Hiroshi Kumigashira and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1063/5.0115384},
doi = {10.1063/5.0115384},
year = {2022},
date = {2022-11-08},
journal = {Applied Physics Letters},
volume = {121},
issue = {19},
pages = {192108},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
高効率エネルギー輸送を拓く超伝導材料の開発

【記事・プレスリリース】
- 排熱を電気に変える高性能熱電素子実現へ (2020.12.2)
- 酸化物に圧力を加えて、熱電変換における電気伝導率と熱起電力のトレードオフ問題を解決 (2021.10.22)
- 金属と絶縁体を重ねて熱電変換電圧を10倍に増大 (2021.12.3)
- セレン化スズ多結晶体の熱電変換性能を30倍に向上 (2022.3.15)
- 従来の常識を覆す発想で酸化物の熱電変換効率を向上 (2023.4.19)
- 過去最高の変換効率を示す毒性元素を含まない熱電材料 (2023.12.27)
【関連論文】
Takayoshi Katase, Seiya Nomoto, Xinyi He, Suguru Kitani, Takashi Honda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
ACS Applied Electronic Materials, vol. 6, iss. 10, pp. 7424–7429, 2024.
@article{nokey,
title = {Simultaneous Realization of Single-Crystal-Like Electron Transport and Strong Phonon Scattering in Polycrystalline SrTiO_{3–x}H_{x}},
author = {Takayoshi Katase and Seiya Nomoto and Xinyi He and Suguru Kitani and Takashi Honda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acsaelm.4c01306},
doi = {10.1021/acsaelm.4c01306},
year = {2024},
date = {2024-09-30},
journal = {ACS Applied Electronic Materials},
volume = {6},
issue = {10},
pages = {7424–7429},
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Chihiro Yamamoto, Xinyi He, Kota Hanzawa, Takayoshi Katase, Masato Sasase, Jun-ichi Yamaura, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Phonon drag thermopower persisting over 200 K in FeSb2 thin film on SrTiO3 single crystal
Applied Physics Letters, vol. 124, iss. 19, pp. 193902, 2024.
@article{nokey,
title = {Phonon drag thermopower persisting over 200 K in FeSb_{2} thin film on SrTiO_{3} single crystal},
author = {Chihiro Yamamoto and Xinyi He and Kota Hanzawa and Takayoshi Katase and Masato Sasase and Jun-ichi Yamaura and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1063/5.0204885},
doi = {10.1063/5.0204885},
year = {2024},
date = {2024-05-06},
journal = {Applied Physics Letters},
volume = {124},
issue = {19},
pages = {193902},
keywords = {},
pubstate = {published},
tppubtype = {article}
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Xinyi He, Shigeru Kimura, Takayoshi Katase, Terumasa Tadano, Satoru Matsuishi, Makoto Minohara, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 11, iss. 10, pp. 2307058, 2023.
@article{nokey,
title = {Inverse-Perovskite Ba_{3}\textit{B}O (\textit{B} = Si and Ge) as a HighPerformance Environmentally Benign Thermoelectric Material with Low Lattice Thermal Conductivity},
author = {Xinyi He and Shigeru Kimura and Takayoshi Katase and Terumasa Tadano and Satoru Matsuishi and Makoto Minohara and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202307058},
doi = {10.1002/advs.202307058},
year = {2023},
date = {2023-12-25},
journal = {Advanced Science},
volume = {11},
issue = {10},
pages = {2307058},
keywords = {},
pubstate = {published},
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Xinyi He, Seiya Nomoto, Takehito Komatsu, Takayoshi Katase, Terumasa Tadano, Suguru Kitani, Hideto Yoshida, Takafumi Yamamoto, Hiroshi Mizoguchi, Keisuke Ide, Hidenori Hiramatsu, Hitoshi Kawaji, Hideo Hosono, Toshio Kamiya
Advanced Functional Materials, vol. 33, iss. 28, pp. 2213144, 2023.
@article{nokey,
title = {Hydride anion substitution boosts thermoelectric performance of polycrystalline SrTiO_{3} via simultaneous realization of reduced thermal conductivity and high electronic conductivity},
author = {Xinyi He and Seiya Nomoto and Takehito Komatsu and Takayoshi Katase and Terumasa Tadano and Suguru Kitani and Hideto Yoshida and Takafumi Yamamoto and Hiroshi Mizoguchi and Keisuke Ide and Hidenori Hiramatsu and Hitoshi Kawaji and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/adfm.202213144},
doi = {10.1002/adfm.202213144},
year = {2023},
date = {2023-04-18},
journal = {Advanced Functional Materials},
volume = {33},
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pages = {2213144},
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Xinyi He, Haoyun Zhang, Takumi Nose, Takayoshi Katase, Terumasa Tadano, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 9, iss. 13, pp. 2105958, 2022.
@article{nokey,
title = {Degenerated Hole Doping and Ultra-Low Lattice Thermal Conductivity in Polycrystalline SnSe by Nonequilibrium Isovalent Te Substitution},
author = {Xinyi He and Haoyun Zhang and Takumi Nose and Takayoshi Katase and Terumasa Tadano and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202105958},
doi = {10.1002/advs.202105958},
year = {2022},
date = {2022-03-08},
journal = {Advanced Science},
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Takayoshi Katase, Xinyi He, Terumasa Tadano, Jan M. Tomczak, Takaki Onozato, Keisuke Ide, Bin Feng, Tetsuya Tohei, Hidenori Hiramatsu, Hiromichi Ohta, Yuichi Ikuhara, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 8, iss. 23, pp. 2102097, 2021.
@article{nokey,
title = {Breaking of thermopower - conductivity trade-off in LaTiO_{3} film around Mott insulator to metal transition},
author = {Takayoshi Katase and Xinyi He and Terumasa Tadano and Jan M. Tomczak and Takaki Onozato and Keisuke Ide and Bin Feng and Tetsuya Tohei and Hidenori Hiramatsu and Hiromichi Ohta and Yuichi Ikuhara and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202102097},
doi = {10.1002/advs.202102097},
year = {2021},
date = {2021-12-08},
journal = {Advanced Science},
volume = {8},
issue = {23},
pages = {2102097},
keywords = {},
pubstate = {published},
tppubtype = {article}
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Masatoshi Kimura, Xinyi He, Takayoshi Katase, Terumasa Tadano, Jan M. Tomczak, Makoto Minohara, Ryotaro Aso, Hideto Yoshida, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Nano Letters, vol. 21, iss. 21, pp. 9240–9246, 2021.
@article{nokey,
title = {Large phonon drag thermopower boosted by massive electrons and phonon leaking in LaAlO_{3}/LaNiO_{3}/LaAlO_{3} heterostructure},
author = {Masatoshi Kimura and Xinyi He and Takayoshi Katase and Terumasa Tadano and Jan M. Tomczak and Makoto Minohara and Ryotaro Aso and Hideto Yoshida and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acs.nanolett.1c03143},
doi = {10.1021/acs.nanolett.1c03143},
year = {2021},
date = {2021-10-28},
journal = {Nano Letters},
volume = {21},
issue = {21},
pages = {9240–9246},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Chihiro Yamamoto, Xinyi He, Takayoshi Katase, Keisuke Ide, Yosuke Goto, Yoshikazu Mizuguchi, Akane Samizo, Makoto Minohara, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Double charge polarity switching in Sb-doped SnSe with switchable substitution sites
Advanced Functional Materials, vol. 31, iss. 8, pp. 2008092, 2020.
@article{nokey,
title = {Double charge polarity switching in Sb-doped SnSe with switchable substitution sites},
author = {Chihiro Yamamoto and Xinyi He and Takayoshi Katase and Keisuke Ide and Yosuke Goto and Yoshikazu Mizuguchi and Akane Samizo and Makoto Minohara and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/adfm.202008092},
doi = {10.1002/adfm.202008092},
year = {2020},
date = {2020-12-01},
journal = {Advanced Functional Materials},
volume = {31},
issue = {8},
pages = {2008092},
keywords = {},
pubstate = {published},
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}
廃熱から電気を作る熱電変換材料の開発
廃熱を電気に変換できる熱電変換技術は、未利用熱エネルギーの有効活用に向けた鍵として期待されています。しかし、従来の熱電材料は、希少で毒性のある重元素が主に使われており、大規模な熱電発電の普及の妨げになっています。
当研究室では、最先端の計算科学と実験を通じて、熱を運ぶ電子とフォノンを巧みに操る材料設計を構築し、環境調和元素からなる高性能熱電材料の開発に挑戦しています。例えば、SrTiO3の多結晶体に水素を添加することで、高性能熱電材料に必要な低い熱伝導率と高い電気出力を両立させ、熱電変換効率を向上させることに成功しました。また、逆ペロブスカイト構造と呼ばれる特殊な結晶構造を持つBa3SiOが、約300°C付近において、毒性元素を一切含まない材料としては最高レベルの熱電変換効率を示す可能性を持つことを見出しています。こうした新材料の開発をさらに深化させ、発電モジュール化を視野に入れた研究を推進します。

【記事・プレスリリース】
- 排熱を電気に変える高性能熱電素子実現へ (2020.12.2)
- 酸化物に圧力を加えて、熱電変換における電気伝導率と熱起電力のトレードオフ問題を解決 (2021.10.22)
- 金属と絶縁体を重ねて熱電変換電圧を10倍に増大 (2021.12.3)
- セレン化スズ多結晶体の熱電変換性能を30倍に向上 (2022.3.15)
- 従来の常識を覆す発想で酸化物の熱電変換効率を向上 (2023.4.19)
- 過去最高の変換効率を示す毒性元素を含まない熱電材料 (2023.12.27)
【関連論文】
Takayoshi Katase, Seiya Nomoto, Xinyi He, Suguru Kitani, Takashi Honda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
ACS Applied Electronic Materials, vol. 6, iss. 10, pp. 7424–7429, 2024.
@article{nokey,
title = {Simultaneous Realization of Single-Crystal-Like Electron Transport and Strong Phonon Scattering in Polycrystalline SrTiO_{3–x}H_{x}},
author = {Takayoshi Katase and Seiya Nomoto and Xinyi He and Suguru Kitani and Takashi Honda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acsaelm.4c01306},
doi = {10.1021/acsaelm.4c01306},
year = {2024},
date = {2024-09-30},
journal = {ACS Applied Electronic Materials},
volume = {6},
issue = {10},
pages = {7424–7429},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Chihiro Yamamoto, Xinyi He, Kota Hanzawa, Takayoshi Katase, Masato Sasase, Jun-ichi Yamaura, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Phonon drag thermopower persisting over 200 K in FeSb2 thin film on SrTiO3 single crystal
Applied Physics Letters, vol. 124, iss. 19, pp. 193902, 2024.
@article{nokey,
title = {Phonon drag thermopower persisting over 200 K in FeSb_{2} thin film on SrTiO_{3} single crystal},
author = {Chihiro Yamamoto and Xinyi He and Kota Hanzawa and Takayoshi Katase and Masato Sasase and Jun-ichi Yamaura and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1063/5.0204885},
doi = {10.1063/5.0204885},
year = {2024},
date = {2024-05-06},
journal = {Applied Physics Letters},
volume = {124},
issue = {19},
pages = {193902},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Xinyi He, Shigeru Kimura, Takayoshi Katase, Terumasa Tadano, Satoru Matsuishi, Makoto Minohara, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 11, iss. 10, pp. 2307058, 2023.
@article{nokey,
title = {Inverse-Perovskite Ba_{3}\textit{B}O (\textit{B} = Si and Ge) as a HighPerformance Environmentally Benign Thermoelectric Material with Low Lattice Thermal Conductivity},
author = {Xinyi He and Shigeru Kimura and Takayoshi Katase and Terumasa Tadano and Satoru Matsuishi and Makoto Minohara and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202307058},
doi = {10.1002/advs.202307058},
year = {2023},
date = {2023-12-25},
journal = {Advanced Science},
volume = {11},
issue = {10},
pages = {2307058},
keywords = {},
pubstate = {published},
tppubtype = {article}
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Xinyi He, Seiya Nomoto, Takehito Komatsu, Takayoshi Katase, Terumasa Tadano, Suguru Kitani, Hideto Yoshida, Takafumi Yamamoto, Hiroshi Mizoguchi, Keisuke Ide, Hidenori Hiramatsu, Hitoshi Kawaji, Hideo Hosono, Toshio Kamiya
Advanced Functional Materials, vol. 33, iss. 28, pp. 2213144, 2023.
@article{nokey,
title = {Hydride anion substitution boosts thermoelectric performance of polycrystalline SrTiO_{3} via simultaneous realization of reduced thermal conductivity and high electronic conductivity},
author = {Xinyi He and Seiya Nomoto and Takehito Komatsu and Takayoshi Katase and Terumasa Tadano and Suguru Kitani and Hideto Yoshida and Takafumi Yamamoto and Hiroshi Mizoguchi and Keisuke Ide and Hidenori Hiramatsu and Hitoshi Kawaji and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/adfm.202213144},
doi = {10.1002/adfm.202213144},
year = {2023},
date = {2023-04-18},
journal = {Advanced Functional Materials},
volume = {33},
issue = {28},
pages = {2213144},
keywords = {},
pubstate = {published},
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Xinyi He, Haoyun Zhang, Takumi Nose, Takayoshi Katase, Terumasa Tadano, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 9, iss. 13, pp. 2105958, 2022.
@article{nokey,
title = {Degenerated Hole Doping and Ultra-Low Lattice Thermal Conductivity in Polycrystalline SnSe by Nonequilibrium Isovalent Te Substitution},
author = {Xinyi He and Haoyun Zhang and Takumi Nose and Takayoshi Katase and Terumasa Tadano and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202105958},
doi = {10.1002/advs.202105958},
year = {2022},
date = {2022-03-08},
journal = {Advanced Science},
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Takayoshi Katase, Xinyi He, Terumasa Tadano, Jan M. Tomczak, Takaki Onozato, Keisuke Ide, Bin Feng, Tetsuya Tohei, Hidenori Hiramatsu, Hiromichi Ohta, Yuichi Ikuhara, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 8, iss. 23, pp. 2102097, 2021.
@article{nokey,
title = {Breaking of thermopower - conductivity trade-off in LaTiO_{3} film around Mott insulator to metal transition},
author = {Takayoshi Katase and Xinyi He and Terumasa Tadano and Jan M. Tomczak and Takaki Onozato and Keisuke Ide and Bin Feng and Tetsuya Tohei and Hidenori Hiramatsu and Hiromichi Ohta and Yuichi Ikuhara and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202102097},
doi = {10.1002/advs.202102097},
year = {2021},
date = {2021-12-08},
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Masatoshi Kimura, Xinyi He, Takayoshi Katase, Terumasa Tadano, Jan M. Tomczak, Makoto Minohara, Ryotaro Aso, Hideto Yoshida, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Nano Letters, vol. 21, iss. 21, pp. 9240–9246, 2021.
@article{nokey,
title = {Large phonon drag thermopower boosted by massive electrons and phonon leaking in LaAlO_{3}/LaNiO_{3}/LaAlO_{3} heterostructure},
author = {Masatoshi Kimura and Xinyi He and Takayoshi Katase and Terumasa Tadano and Jan M. Tomczak and Makoto Minohara and Ryotaro Aso and Hideto Yoshida and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acs.nanolett.1c03143},
doi = {10.1021/acs.nanolett.1c03143},
year = {2021},
date = {2021-10-28},
journal = {Nano Letters},
volume = {21},
issue = {21},
pages = {9240–9246},
keywords = {},
pubstate = {published},
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}
Chihiro Yamamoto, Xinyi He, Takayoshi Katase, Keisuke Ide, Yosuke Goto, Yoshikazu Mizuguchi, Akane Samizo, Makoto Minohara, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Double charge polarity switching in Sb-doped SnSe with switchable substitution sites
Advanced Functional Materials, vol. 31, iss. 8, pp. 2008092, 2020.
@article{nokey,
title = {Double charge polarity switching in Sb-doped SnSe with switchable substitution sites},
author = {Chihiro Yamamoto and Xinyi He and Takayoshi Katase and Keisuke Ide and Yosuke Goto and Yoshikazu Mizuguchi and Akane Samizo and Makoto Minohara and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/adfm.202008092},
doi = {10.1002/adfm.202008092},
year = {2020},
date = {2020-12-01},
journal = {Advanced Functional Materials},
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issue = {8},
pages = {2008092},
keywords = {},
pubstate = {published},
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断熱から放熱まで:熱制御材料の開発
電子機器や自動車、エネルギー変換デバイスなどの高性能化に伴い、効率的な熱マネジメント技術の重要性がますます高まっています。当研究室では、結晶構造の次元性変化を変化させる新物質を開発し、温度によって断熱と放熱を切り替える熱制御材料を実証してきました。最近では、効率よく熱を放出できる超高熱伝導材料の開発も推進し、断熱から放熱まで熱の流れを自在に操る革新的な熱制御材料の開発を目指しています。

【記事・プレスリリース】
- 排熱を電気に変える高性能熱電素子実現へ (2020.12.2)
- 酸化物に圧力を加えて、熱電変換における電気伝導率と熱起電力のトレードオフ問題を解決 (2021.10.22)
- 金属と絶縁体を重ねて熱電変換電圧を10倍に増大 (2021.12.3)
- セレン化スズ多結晶体の熱電変換性能を30倍に向上 (2022.3.15)
- 従来の常識を覆す発想で酸化物の熱電変換効率を向上 (2023.4.19)
- 過去最高の変換効率を示す毒性元素を含まない熱電材料 (2023.12.27)
【関連論文】
Takayoshi Katase, Seiya Nomoto, Xinyi He, Suguru Kitani, Takashi Honda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
ACS Applied Electronic Materials, vol. 6, iss. 10, pp. 7424–7429, 2024.
@article{nokey,
title = {Simultaneous Realization of Single-Crystal-Like Electron Transport and Strong Phonon Scattering in Polycrystalline SrTiO_{3–x}H_{x}},
author = {Takayoshi Katase and Seiya Nomoto and Xinyi He and Suguru Kitani and Takashi Honda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acsaelm.4c01306},
doi = {10.1021/acsaelm.4c01306},
year = {2024},
date = {2024-09-30},
journal = {ACS Applied Electronic Materials},
volume = {6},
issue = {10},
pages = {7424–7429},
keywords = {},
pubstate = {published},
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Chihiro Yamamoto, Xinyi He, Kota Hanzawa, Takayoshi Katase, Masato Sasase, Jun-ichi Yamaura, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Phonon drag thermopower persisting over 200 K in FeSb2 thin film on SrTiO3 single crystal
Applied Physics Letters, vol. 124, iss. 19, pp. 193902, 2024.
@article{nokey,
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Xinyi He, Shigeru Kimura, Takayoshi Katase, Terumasa Tadano, Satoru Matsuishi, Makoto Minohara, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 11, iss. 10, pp. 2307058, 2023.
@article{nokey,
title = {Inverse-Perovskite Ba_{3}\textit{B}O (\textit{B} = Si and Ge) as a HighPerformance Environmentally Benign Thermoelectric Material with Low Lattice Thermal Conductivity},
author = {Xinyi He and Shigeru Kimura and Takayoshi Katase and Terumasa Tadano and Satoru Matsuishi and Makoto Minohara and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
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Xinyi He, Seiya Nomoto, Takehito Komatsu, Takayoshi Katase, Terumasa Tadano, Suguru Kitani, Hideto Yoshida, Takafumi Yamamoto, Hiroshi Mizoguchi, Keisuke Ide, Hidenori Hiramatsu, Hitoshi Kawaji, Hideo Hosono, Toshio Kamiya
Advanced Functional Materials, vol. 33, iss. 28, pp. 2213144, 2023.
@article{nokey,
title = {Hydride anion substitution boosts thermoelectric performance of polycrystalline SrTiO_{3} via simultaneous realization of reduced thermal conductivity and high electronic conductivity},
author = {Xinyi He and Seiya Nomoto and Takehito Komatsu and Takayoshi Katase and Terumasa Tadano and Suguru Kitani and Hideto Yoshida and Takafumi Yamamoto and Hiroshi Mizoguchi and Keisuke Ide and Hidenori Hiramatsu and Hitoshi Kawaji and Hideo Hosono and Toshio Kamiya},
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Xinyi He, Haoyun Zhang, Takumi Nose, Takayoshi Katase, Terumasa Tadano, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 9, iss. 13, pp. 2105958, 2022.
@article{nokey,
title = {Degenerated Hole Doping and Ultra-Low Lattice Thermal Conductivity in Polycrystalline SnSe by Nonequilibrium Isovalent Te Substitution},
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Takayoshi Katase, Xinyi He, Terumasa Tadano, Jan M. Tomczak, Takaki Onozato, Keisuke Ide, Bin Feng, Tetsuya Tohei, Hidenori Hiramatsu, Hiromichi Ohta, Yuichi Ikuhara, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 8, iss. 23, pp. 2102097, 2021.
@article{nokey,
title = {Breaking of thermopower - conductivity trade-off in LaTiO_{3} film around Mott insulator to metal transition},
author = {Takayoshi Katase and Xinyi He and Terumasa Tadano and Jan M. Tomczak and Takaki Onozato and Keisuke Ide and Bin Feng and Tetsuya Tohei and Hidenori Hiramatsu and Hiromichi Ohta and Yuichi Ikuhara and Hideo Hosono and Toshio Kamiya},
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Masatoshi Kimura, Xinyi He, Takayoshi Katase, Terumasa Tadano, Jan M. Tomczak, Makoto Minohara, Ryotaro Aso, Hideto Yoshida, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Nano Letters, vol. 21, iss. 21, pp. 9240–9246, 2021.
@article{nokey,
title = {Large phonon drag thermopower boosted by massive electrons and phonon leaking in LaAlO_{3}/LaNiO_{3}/LaAlO_{3} heterostructure},
author = {Masatoshi Kimura and Xinyi He and Takayoshi Katase and Terumasa Tadano and Jan M. Tomczak and Makoto Minohara and Ryotaro Aso and Hideto Yoshida and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
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Chihiro Yamamoto, Xinyi He, Takayoshi Katase, Keisuke Ide, Yosuke Goto, Yoshikazu Mizuguchi, Akane Samizo, Makoto Minohara, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Double charge polarity switching in Sb-doped SnSe with switchable substitution sites
Advanced Functional Materials, vol. 31, iss. 8, pp. 2008092, 2020.
@article{nokey,
title = {Double charge polarity switching in Sb-doped SnSe with switchable substitution sites},
author = {Chihiro Yamamoto and Xinyi He and Takayoshi Katase and Keisuke Ide and Yosuke Goto and Yoshikazu Mizuguchi and Akane Samizo and Makoto Minohara and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
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非平衡・薄膜ヘテロ構造を利用した新機能の探索
熱力学的な安定相ではない非平衡構造を安定化させたり、原子層で人工的な界面を形成したりすることで、天然材料では実現できない、全く新しい物性や機能が発現します。当研究室では、薄膜成長技術を駆使した非平衡相やヘテロ接合の設計により、新しい電子・光・熱機能の探索を進めています。その一例として、1 nmまで薄くしたLaNiO3超薄膜を絶縁体LaAlO3で挟み込んだ人工構造を作製し、界面フォノンが電子を引っ張る「フォノンドラッグ効果」によって熱起電力が10倍増加する現象を発見しました。また、2D層状SnSeと3D岩塩型PbSeの相境界を非平衡状態で安定化し、温度変化による2D⇔3D構造の可逆転移と5桁を超える巨大な電気抵抗変化を実現しています。安定相物質では成し得ない性能や新機能を持つ革新材料とデバイスの創出を目指しています。

【記事・プレスリリース】
- 排熱を電気に変える高性能熱電素子実現へ (2020.12.2)
- 酸化物に圧力を加えて、熱電変換における電気伝導率と熱起電力のトレードオフ問題を解決 (2021.10.22)
- 金属と絶縁体を重ねて熱電変換電圧を10倍に増大 (2021.12.3)
- セレン化スズ多結晶体の熱電変換性能を30倍に向上 (2022.3.15)
- 従来の常識を覆す発想で酸化物の熱電変換効率を向上 (2023.4.19)
- 過去最高の変換効率を示す毒性元素を含まない熱電材料 (2023.12.27)
【関連論文】
Takayoshi Katase, Seiya Nomoto, Xinyi He, Suguru Kitani, Takashi Honda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
ACS Applied Electronic Materials, vol. 6, iss. 10, pp. 7424–7429, 2024.
@article{nokey,
title = {Simultaneous Realization of Single-Crystal-Like Electron Transport and Strong Phonon Scattering in Polycrystalline SrTiO_{3–x}H_{x}},
author = {Takayoshi Katase and Seiya Nomoto and Xinyi He and Suguru Kitani and Takashi Honda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acsaelm.4c01306},
doi = {10.1021/acsaelm.4c01306},
year = {2024},
date = {2024-09-30},
journal = {ACS Applied Electronic Materials},
volume = {6},
issue = {10},
pages = {7424–7429},
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pubstate = {published},
tppubtype = {article}
}
Chihiro Yamamoto, Xinyi He, Kota Hanzawa, Takayoshi Katase, Masato Sasase, Jun-ichi Yamaura, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Phonon drag thermopower persisting over 200 K in FeSb2 thin film on SrTiO3 single crystal
Applied Physics Letters, vol. 124, iss. 19, pp. 193902, 2024.
@article{nokey,
title = {Phonon drag thermopower persisting over 200 K in FeSb_{2} thin film on SrTiO_{3} single crystal},
author = {Chihiro Yamamoto and Xinyi He and Kota Hanzawa and Takayoshi Katase and Masato Sasase and Jun-ichi Yamaura and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1063/5.0204885},
doi = {10.1063/5.0204885},
year = {2024},
date = {2024-05-06},
journal = {Applied Physics Letters},
volume = {124},
issue = {19},
pages = {193902},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Xinyi He, Shigeru Kimura, Takayoshi Katase, Terumasa Tadano, Satoru Matsuishi, Makoto Minohara, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 11, iss. 10, pp. 2307058, 2023.
@article{nokey,
title = {Inverse-Perovskite Ba_{3}\textit{B}O (\textit{B} = Si and Ge) as a HighPerformance Environmentally Benign Thermoelectric Material with Low Lattice Thermal Conductivity},
author = {Xinyi He and Shigeru Kimura and Takayoshi Katase and Terumasa Tadano and Satoru Matsuishi and Makoto Minohara and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202307058},
doi = {10.1002/advs.202307058},
year = {2023},
date = {2023-12-25},
journal = {Advanced Science},
volume = {11},
issue = {10},
pages = {2307058},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Xinyi He, Seiya Nomoto, Takehito Komatsu, Takayoshi Katase, Terumasa Tadano, Suguru Kitani, Hideto Yoshida, Takafumi Yamamoto, Hiroshi Mizoguchi, Keisuke Ide, Hidenori Hiramatsu, Hitoshi Kawaji, Hideo Hosono, Toshio Kamiya
Advanced Functional Materials, vol. 33, iss. 28, pp. 2213144, 2023.
@article{nokey,
title = {Hydride anion substitution boosts thermoelectric performance of polycrystalline SrTiO_{3} via simultaneous realization of reduced thermal conductivity and high electronic conductivity},
author = {Xinyi He and Seiya Nomoto and Takehito Komatsu and Takayoshi Katase and Terumasa Tadano and Suguru Kitani and Hideto Yoshida and Takafumi Yamamoto and Hiroshi Mizoguchi and Keisuke Ide and Hidenori Hiramatsu and Hitoshi Kawaji and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/adfm.202213144},
doi = {10.1002/adfm.202213144},
year = {2023},
date = {2023-04-18},
journal = {Advanced Functional Materials},
volume = {33},
issue = {28},
pages = {2213144},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Xinyi He, Haoyun Zhang, Takumi Nose, Takayoshi Katase, Terumasa Tadano, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 9, iss. 13, pp. 2105958, 2022.
@article{nokey,
title = {Degenerated Hole Doping and Ultra-Low Lattice Thermal Conductivity in Polycrystalline SnSe by Nonequilibrium Isovalent Te Substitution},
author = {Xinyi He and Haoyun Zhang and Takumi Nose and Takayoshi Katase and Terumasa Tadano and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202105958},
doi = {10.1002/advs.202105958},
year = {2022},
date = {2022-03-08},
journal = {Advanced Science},
volume = {9},
issue = {13},
pages = {2105958},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Takayoshi Katase, Xinyi He, Terumasa Tadano, Jan M. Tomczak, Takaki Onozato, Keisuke Ide, Bin Feng, Tetsuya Tohei, Hidenori Hiramatsu, Hiromichi Ohta, Yuichi Ikuhara, Hideo Hosono, Toshio Kamiya
Advanced Science, vol. 8, iss. 23, pp. 2102097, 2021.
@article{nokey,
title = {Breaking of thermopower - conductivity trade-off in LaTiO_{3} film around Mott insulator to metal transition},
author = {Takayoshi Katase and Xinyi He and Terumasa Tadano and Jan M. Tomczak and Takaki Onozato and Keisuke Ide and Bin Feng and Tetsuya Tohei and Hidenori Hiramatsu and Hiromichi Ohta and Yuichi Ikuhara and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/advs.202102097},
doi = {10.1002/advs.202102097},
year = {2021},
date = {2021-12-08},
journal = {Advanced Science},
volume = {8},
issue = {23},
pages = {2102097},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Masatoshi Kimura, Xinyi He, Takayoshi Katase, Terumasa Tadano, Jan M. Tomczak, Makoto Minohara, Ryotaro Aso, Hideto Yoshida, Keisuke Ide, Shigenori Ueda, Hidenori Hiramatsu, Hiroshi Kumigashira, Hideo Hosono, Toshio Kamiya
Nano Letters, vol. 21, iss. 21, pp. 9240–9246, 2021.
@article{nokey,
title = {Large phonon drag thermopower boosted by massive electrons and phonon leaking in LaAlO_{3}/LaNiO_{3}/LaAlO_{3} heterostructure},
author = {Masatoshi Kimura and Xinyi He and Takayoshi Katase and Terumasa Tadano and Jan M. Tomczak and Makoto Minohara and Ryotaro Aso and Hideto Yoshida and Keisuke Ide and Shigenori Ueda and Hidenori Hiramatsu and Hiroshi Kumigashira and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1021/acs.nanolett.1c03143},
doi = {10.1021/acs.nanolett.1c03143},
year = {2021},
date = {2021-10-28},
journal = {Nano Letters},
volume = {21},
issue = {21},
pages = {9240–9246},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Chihiro Yamamoto, Xinyi He, Takayoshi Katase, Keisuke Ide, Yosuke Goto, Yoshikazu Mizuguchi, Akane Samizo, Makoto Minohara, Shigenori Ueda, Hidenori Hiramatsu, Hideo Hosono, Toshio Kamiya
Double charge polarity switching in Sb-doped SnSe with switchable substitution sites
Advanced Functional Materials, vol. 31, iss. 8, pp. 2008092, 2020.
@article{nokey,
title = {Double charge polarity switching in Sb-doped SnSe with switchable substitution sites},
author = {Chihiro Yamamoto and Xinyi He and Takayoshi Katase and Keisuke Ide and Yosuke Goto and Yoshikazu Mizuguchi and Akane Samizo and Makoto Minohara and Shigenori Ueda and Hidenori Hiramatsu and Hideo Hosono and Toshio Kamiya},
url = {https://doi.org/10.1002/adfm.202008092},
doi = {10.1002/adfm.202008092},
year = {2020},
date = {2020-12-01},
journal = {Advanced Functional Materials},
volume = {31},
issue = {8},
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